Reductive amination using cobalt-based nanoparticles for synthesis of amines.


Journal

Nature protocols
ISSN: 1750-2799
Titre abrégé: Nat Protoc
Pays: England
ID NLM: 101284307

Informations de publication

Date de publication:
04 2020
Historique:
received: 14 02 2019
accepted: 21 10 2019
pubmed: 24 3 2020
medline: 18 4 2020
entrez: 24 3 2020
Statut: ppublish

Résumé

Reductive aminations are an essential class of reactions widely applied for the preparation of different kinds of amines, as well as a number of pharmaceuticals and industrially relevant compounds. In such reactions, carbonyl compounds (aldehydes, ketones) react with ammonia or amines in the presence of a reducing agent and form corresponding amines. Common catalysts used for reductive aminations, especially for the synthesis of primary amines, are based on precious metals or Raney nickel. However, their drawbacks and limited applicability inspired us to look for alternative catalysts. The development of base-metal nanostructured catalysts is highly preferable and is crucial to the advancement of sustainable and cost-effective reductive amination processes. In this protocol, we describe the preparation of carbon-supported cobalt-based nanoparticles as efficient and practical catalysts for synthesis of different kinds of amines by reductive aminations. Template synthesis of a cobalt-triethylenediamine-terephthalic acid metal-organic framework on carbon and subsequent pyrolysis to remove the organic template resulted in the formation of supported single cobalt atoms and nanoparticles. Applying these catalysts, we have synthesized structurally diverse benzylic, aliphatic and heterocyclic primary, secondary and tertiary amines, including pharmaceutically relevant products, starting from inexpensive and easily accessible carbonyl compounds with ammonia, nitro compounds or amines and molecular hydrogen. To prepare this cobalt-based catalyst takes 26 h, and the reported catalytic reductive amination reactions can be carried out within 18-28 h.

Identifiants

pubmed: 32203487
doi: 10.1038/s41596-019-0258-z
pii: 10.1038/s41596-019-0258-z
doi:

Substances chimiques

Amines 0
Metal-Organic Frameworks 0
Cobalt 3G0H8C9362

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

1313-1337

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Auteurs

Kathiravan Murugesan (K)

Leibniz-Institut für Katalyse e.V. an der Universität Rostock, Rostock, Germany.

Vishwas G Chandrashekhar (VG)

Leibniz-Institut für Katalyse e.V. an der Universität Rostock, Rostock, Germany.

Thirusangumurugan Senthamarai (T)

Leibniz-Institut für Katalyse e.V. an der Universität Rostock, Rostock, Germany.

Rajenahally V Jagadeesh (RV)

Leibniz-Institut für Katalyse e.V. an der Universität Rostock, Rostock, Germany. jagadeesh.rajenahally@catalysis.de.

Matthias Beller (M)

Leibniz-Institut für Katalyse e.V. an der Universität Rostock, Rostock, Germany. matthias.beller@catalysis.de.

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