Studying the excited electronic states of guanine rich DNA quadruplexes by quantum mechanical methods: main achievements and perspectives.


Journal

Photochemical & photobiological sciences : Official journal of the European Photochemistry Association and the European Society for Photobiology
ISSN: 1474-9092
Titre abrégé: Photochem Photobiol Sci
Pays: England
ID NLM: 101124451

Informations de publication

Date de publication:
15 Apr 2020
Historique:
pubmed: 8 4 2020
medline: 15 12 2020
entrez: 8 4 2020
Statut: ppublish

Résumé

The main insights into the photoactivated dynamics of guanine quadruplexes (G4s) recently provided by quantum mechanical computations are concisely reviewed here. The experimental steady state absorption and circular dichroism spectra of different topologies can be reproduced and assigned. After light absorption from excited states delocalized over multiple bases, the most important decay pathways involve localization of the excitation over a single base or on two stacked guanines, excimers with different degrees of charge transfer character. Two main photochemical reactions are discussed. One involves the photodimerization of two stacked guanine bases on the 'neutral' excimer path. The other, ionization of guanine, which triggers deprotonation of the resulting cation to form (G-H2)˙ and (G-H1)˙ radicals. Both the static and dynamical properties of G4 excited states are ruled by their topology and modulated by the inner coordinated metal ions.

Identifiants

pubmed: 32255446
doi: 10.1039/d0pp00065e
pii: 10.1039/d0pp00065e
doi:

Substances chimiques

Guanine 5Z93L87A1R
DNA 9007-49-2

Types de publication

Journal Article Review

Langues

eng

Sous-ensembles de citation

IM

Pagination

436-444

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Auteurs

Lara Martínez-Fernández (L)

Departamento de Química, Facultad de Ciencias, Modulo 13 Universidad Autónoma de Madrid, Campus de Excelencia UAM-CSIC Cantoblanco, Madrid, 28049, Spain.
IADCHEM, Institute for Advanced Research in Chemistry, Universidad Autónoma de Madrid, Cantoblanco, Madrid, 28049, Spain.

Luciana Esposito (L)

Istituto di Biostrutture e Bioimmagini, CNR, Via Mezzocannone 16, Napoli, I-80134, Italy.

Roberto Improta (R)

Istituto di Biostrutture e Bioimmagini, CNR, Via Mezzocannone 16, Napoli, I-80134, Italy. robimp@unina.it.

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