Sulfation modulates the targeting properties of hyaluronic acid to P-selectin and CD44.

CD44 P-selectin dual target hyaluronic acid near infrared

Journal

ACS biomaterials science & engineering
ISSN: 2373-9878
Titre abrégé: ACS Biomater Sci Eng
Pays: United States
ID NLM: 101654670

Informations de publication

Date de publication:
08 06 2020
Historique:
entrez: 4 7 2020
pubmed: 4 7 2020
medline: 4 7 2020
Statut: ppublish

Résumé

Many targeting strategies can be employed to direct nanoparticles to tumors for imaging and therapy. However, tumors display a dynamic, heterogeneous microenvironment that undergoes spatiotemporal changes, including the expression of targetable cell-surface biomarkers. Here, we develop a nanoparticle system to effectively target two receptors overexpressed in the microenvironment of aggressive tumors. Hyaluronic acid (HA) was regioselectivity modified using a multi-step synthetic approach to alter binding specificities for CD44 and P-selectin to tumor cell interaction. The dual-targeting strategy utilizes sulfate modifications on HA that targets P-selectin, in addition to native targeting of CD44, which exploits spatiotemporal alterations in the expression patterns of these two receptors in cancer sites. Using biophysical characterization and

Identifiants

pubmed: 32617404
doi: 10.1021/acsbiomaterials.0c00115
pmc: PMC7331950
mid: NIHMS1592040
doi:

Substances chimiques

P-Selectin 0
Hyaluronic Acid 9004-61-9

Types de publication

Journal Article Research Support, N.I.H., Extramural Research Support, Non-U.S. Gov't

Langues

eng

Pagination

3585-3598

Subventions

Organisme : NIGMS NIH HHS
ID : P20 GM103427
Pays : United States
Organisme : NCI NIH HHS
ID : P30 CA036727
Pays : United States
Organisme : NIGMS NIH HHS
ID : P30 GM106397
Pays : United States
Organisme : NIBIB NIH HHS
ID : R01 EB019449
Pays : United States

Déclaration de conflit d'intérêts

The authors declare no competing financial interest.

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Auteurs

Deep S Bhattacharya (DS)

Department of Pharmaceutical Sciences, University of Nebraska Medical Center, Omaha, NE 68198, United States.

Denis Svechkarev (D)

Department of Pharmaceutical Sciences, University of Nebraska Medical Center, Omaha, NE 68198, United States.

Aishwarya Bapat (A)

Department of Pharmaceutical Sciences, University of Nebraska Medical Center, Omaha, NE 68198, United States.

Prathamesh Patil (P)

Eppley Institute for Research in Cancer and Allied Diseases, University of Nebraska Medical Center, Omaha, NE 68198, United States.

Michael A Hollingsworth (MA)

Eppley Institute for Research in Cancer and Allied Diseases, University of Nebraska Medical Center, Omaha, NE 68198, United States.
Fred and Pamela Buffett Cancer Center, University of Nebraska Medical Center, Omaha, NE 68198, United States.

Aaron M Mohs (AM)

Department of Pharmaceutical Sciences, University of Nebraska Medical Center, Omaha, NE 68198, United States.
Fred and Pamela Buffett Cancer Center, University of Nebraska Medical Center, Omaha, NE 68198, United States.
Department of Biochemistry and Molecular Biology, University of Nebraska Medical Center, Omaha, NE 68198.

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Classifications MeSH