Bioinspired Dopamine/Mucin Coatings Provide Lubricity, Wear Protection, and Cell-Repellent Properties for Medical Applications.

anti-biofouling friction implants molecular double-layers wear protection

Journal

Advanced healthcare materials
ISSN: 2192-2659
Titre abrégé: Adv Healthc Mater
Pays: Germany
ID NLM: 101581613

Informations de publication

Date de publication:
02 2021
Historique:
received: 16 05 2020
revised: 09 08 2020
pubmed: 18 9 2020
medline: 15 5 2021
entrez: 17 9 2020
Statut: ppublish

Résumé

Even though medical devices have improved a lot over the past decades, there are still issues regarding their anti-biofouling properties and tribological performance, and both aspects contribute to the short- and long-term failure of these devices. Coating these devices with a biocompatible layer that reduces friction, wear, and biofouling at the same time would be a promising strategy to address these issues. Inspired by the adhesion mechanism employed by mussels, here, dopamine is made use of to immobilize lubricious mucin macromolecules onto both manufactured commercial materials and real medical devices. It is shown that purified mucins successfully adsorb onto a dopamine pre-coated substrate, and that this double-layer is stable toward mechanical challenges and storage in aqueous solutions. Moreover, the results indicate that the dopamine/mucin double-layer decreases friction (especially in the boundary lubrication regime), reduces wear damage, and provides anti-biofouling properties. The results obtained in this study show that such dopamine/mucin double-layer coatings can be powerful candidates for improving the surface properties of medical devices such as catheters, stents, and blood vessel substitutes.

Identifiants

pubmed: 32940004
doi: 10.1002/adhm.202000831
doi:

Substances chimiques

Mucins 0
Dopamine VTD58H1Z2X

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2000831

Informations de copyright

© 2020 The Authors. Published by Wiley-VCH GmbH.

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Auteurs

Jian Song (J)

Department of Mechanical Engineering and Munich School of Bioengineering, Technical University of Munich, 85748, Garching, Germany.

Theresa M Lutz (TM)

Department of Mechanical Engineering and Munich School of Bioengineering, Technical University of Munich, 85748, Garching, Germany.

Nora Lang (N)

Department of Pediatric Cardiology and Congenital Heart Disease, German Heart Center Munich, Technical University of Munich, 80636, Munich, Germany.

Oliver Lieleg (O)

Department of Mechanical Engineering and Munich School of Bioengineering, Technical University of Munich, 85748, Garching, Germany.

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