Structure of the O-Antigen and the Lipid A from the Lipopolysaccharide of Fusobacterium nucleatum ATCC 51191.


Journal

Chembiochem : a European journal of chemical biology
ISSN: 1439-7633
Titre abrégé: Chembiochem
Pays: Germany
ID NLM: 100937360

Informations de publication

Date de publication:
06 04 2021
Historique:
revised: 14 11 2020
received: 31 10 2020
pubmed: 17 11 2020
medline: 18 11 2021
entrez: 16 11 2020
Statut: ppublish

Résumé

Fusobacterium nucleatum is a common member of the oral microbiota. However, this symbiont has been found to play an active role in disease development. As a Gram-negative bacterium, F. nucleatum has a protective outer membrane layer whose external leaflet is mainly composed of lipopolysaccharides (LPSs). LPSs play a crucial role in the interaction between bacteria and the host immune system. Here, we characterised the structure of the O-antigen and lipid A from F. nucleatum ssp. animalis ATCC 51191 by using a combination of GC-MS, MALDI and NMR techniques. The results revealed a novel repeat of the O-antigen structure of the LPS, [→4)-β-d-GlcpNAcA-(1→4)-β-d-GlcpNAc3NAlaA-(1→3)-α-d-FucpNAc4NR-(1→], (R=acetylated 60 %), and a bis-phosphorylated hexa-acylated lipid A moiety. Taken together these data showed that F. nucleatum ATCC 51191 has a distinct LPS which might differentially influence recognition by immune cells.

Identifiants

pubmed: 33197108
doi: 10.1002/cbic.202000751
pmc: PMC8048906
doi:

Substances chimiques

Lipid A 0
Lipopolysaccharides 0
O Antigens 0

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

1252-1260

Subventions

Organisme : UniNA
Organisme : Compagnia di San Paolo
Organisme : Biotechnology and Biological Sciences Research Council
ID : BBS/E/F/00044452
Pays : United Kingdom
Organisme : BBSRC Institute Strategic Programme Grant Gut Microbes and Health
ID : BB/R012490/1

Informations de copyright

© 2020 The Authors. ChemBioChem published by Wiley-VCH GmbH.

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Auteurs

Pilar Garcia-Vello (P)

Departmentof Chemical Sciences, University of Naples Federico II, Via Cinthia, 26, 80126, Napoli, NA, Italy.

Flaviana Di Lorenzo (F)

Departmentof Chemical Sciences, University of Naples Federico II, Via Cinthia, 26, 80126, Napoli, NA, Italy.

Dimitra Lamprinaki (D)

Gut Microbes & Health Institute Strategic Programme, Quadram Institute Bioscience, Rosalind Franklin Road, Norwich Research Park, Norwich, NR4 7UQ, UK.

Anna Notaro (A)

Departmentof Chemical Sciences, University of Naples Federico II, Via Cinthia, 26, 80126, Napoli, NA, Italy.

Immacolata Speciale (I)

Department of Agricultural Sciences, University of Naples Federico II, Via Università, 100, 80055, Portici NA, Italy.

Antonio Molinaro (A)

Departmentof Chemical Sciences, University of Naples Federico II, Via Cinthia, 26, 80126, Napoli, NA, Italy.

Nathalie Juge (N)

Gut Microbes & Health Institute Strategic Programme, Quadram Institute Bioscience, Rosalind Franklin Road, Norwich Research Park, Norwich, NR4 7UQ, UK.

Cristina De Castro (C)

Department of Agricultural Sciences, University of Naples Federico II, Via Università, 100, 80055, Portici NA, Italy.

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Classifications MeSH