Formation of Novel Octuplex DNA Molecules from Guanine Quadruplexes.

DNA nanoelectronics guanine octuplex (G8-DNA) guanine quadruplex (G4-DNA)

Journal

Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358

Informations de publication

Date de publication:
Feb 2021
Historique:
received: 12 10 2020
revised: 14 12 2020
pubmed: 22 1 2021
medline: 7 10 2021
entrez: 21 1 2021
Statut: ppublish

Résumé

Guanine quadruplex (G4)-DNA structures have sparked the interest of many scientists due to their important biological roles and their potential use in molecular nanoelectronics and nanotechnology. The high guanine content in G4-DNA endows it with mechanical stability, robustness, and improved charge transport properties-attractive attributes for a molecular nanowire. The self-driven formation of a novel G4-DNA-based nanostructure, coined guanine octuplex (G8)-DNA, is reported herein. Atomic force microscopy and scanning tunneling microscopy characterization of this molecule reveal its organized coiled-coil structure, which is found to be stable under different temperatures and surrounding conditions. G8-DNA exhibits enhanced stiffness, mechanical and thermodynamic stability when compared to its parent G4-DNA. These, along with its high guanine content, make G8-DNA a compelling new molecule, and a highly prospective candidate for molecular nanoelectronics.

Identifiants

pubmed: 33475220
doi: 10.1002/adma.202006932
doi:

Substances chimiques

DNA 9007-49-2

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2006932

Subventions

Organisme : Israel Science Foundation
ID : 1589/14
Organisme : Israel Science Foundation
ID : 2556/17
Organisme : Ministry of Science & Technology, Israel
ID : 3-16840

Informations de copyright

© 2021 Wiley-VCH GmbH.

Références

D. Varshney, J. Spiegel, K. Zyner, D. Tannahill, S. Balasubramanian, Nat. Rev. Mol. Cell Biol. 2020, 21, 459.
R. Hänsel-Hertsch, M. Di Antonio, S. Balasubramanian, Nat. Rev. Mol. Cell Biol. 2017, 18, 279.
S. Neidle, Nat. Rev. Chem. 2017, 1, 0041.
R. Hänsel-Hertsch, D. Beraldi, S. V. Lensing, G. Marsico, K. Zyner, A. Parry, M. Di Antonio, J. Pike, H. Kimura, M. Narita, Nat. Genet. 2016, 48, 1267.
H. Cohen, T. Sapir, N. Borovok, T. Molotsky, R. Di Felice, A. B. Kotlyar, D. Porath, Nano Lett. 2007, 7, 981.
S. P. Liu, S. H. Weisbrod, Z. Tang, A. Marx, E. Scheer, A. Erbe, Angew. Chem., Int. Ed. 2010, 49, 3313.
G. I. Livshits, A. Stern, D. Rotem, N. Borovok, G. Eidelshtein, A. Migliore, E. Penzo, S. J. Wind, R. Di Felice, S. S. Skourtis, Nat. Nanotechnol. 2014, 9, 1040.
J. T. Davis, Angew. Chem., Int. Ed. 2004, 43, 668.
Y. Li, C. Wang, Y. Zhu, X. Zhou, Y. Xiang, M. He, S. Zeng, Biosens. Bioelectron. 2017, 89, 758.
Y. C. Huang, D. Sen, Angew. Chem. 2014, 126, 14279.
Z. F. Gao, Y. L. Huang, W. Ren, H. Q. Luo, N. B. Li, Biosens. Bioelectron. 2016, 78, 351.
C. Schaffitzel, I. Berger, J. Postberg, J. Hanes, H. J. Lipps, A. Plückthun, Proc. Natl. Acad. Sci. USA 2001, 98, 8572.
K. Paeschke, T. Simonsson, J. Postberg, D. Rhodes, H. J. Lipps, Nat. Struct. Mol. Biol. 2005, 12, 847.
N. Borovok, N. Iram, D. Zikich, J. Ghabboun, G. I. Livshits, D. Porath, A. B. Kotlyar, Nucleic Acids Res. 2008, 36, 5050.
N. Borovok, T. Molotsky, J. Ghabboun, D. Porath, A. Kotlyar, Anal. Biochem. 2008, 374, 71.
A. B. Kotlyar, N. Borovok, T. Molotsky, H. Cohen, E. Shapir, D. Porath, Long, Adv. Mater. 2005, 17, 1901.
M. L. Bochman, K. Paeschke, V. A. Zakian, Nat. Rev. Genet. 2012, 13, 770.
J. R. Williamson, M. Raghuraman, T. R. Cech, Cell 1989, 59, 871.
W. D. Wilson, H. Sugiyama, First International Meeting on Quadruplex DNA, ACS Publications, Washington, D.C., USA 2007.
H. M. Wong, L. Payet, J. L. Huppert, Curr. Opin. Mol. Ther 2009, 11, 146.
E. Protozanova, R. B. Macgregor, Biochemistry 1996, 35, 16638.
L. A. Yatsunyk, O. Pietrement, D. Albrecht, P. L. T. Tran, D. Renciuk, H. Sugiyama, J.-M. Arbona, J.-P. Aimé, J.-L. Mergny, ACS Nano 2013, 7, 5701.
J.-L. Mergny, A.-T. Phan, L. Lacroix, FEBS Lett. 1998, 435, 74.
A. N. Lane, J. B. Chaires, R. D. Gray, J. O. Trent, Nucleic Acids Res. 2008, 36, 5482.
P. A. Rachwal, T. Brown, K. R. Fox, FEBS Lett. 2007, 581, 1657.
A. Bugaut, S. Balasubramanian, Biochemistry 2008, 47, 689.
N. Hush, A. S. Cheung, Chem. Phys. Lett. 1975, 34, 11.
A. A. Voityuk, J. Jortner, M. Bixon, N. Rösch, Chem. Phys. Lett. 2000, 324, 430.
A. A. Voityuk, N. Rösch, M. Bixon, J. Jortner, J. Phys. Chem. B 2000, 104, 9740.
M. Bixon, B. Giese, S. Wessely, T. Langenbacher, M. E. Michel-Beyerle, J. Jortner, Proc. Natl. Acad. Sci. USA 1999, 96, 11713.
P. B. Woiczikowski, T. Kubař, R. Gutiérrez, G. Cuniberti, M. Elstner, J. Chem. Phys. 2010, 133, 035103.
R. Zhuravel, A. Stern, N. Fardian-Melamed, G. Eidelshtein, L. Katrivas, D. Rotem, A. B. Kotlyar, D. Porath, Adv. Mater. 2018, 30, 1706984.
A. Kotlyar, N. Borovok, T. Molotsky, D. Klinov, B. Dwir, E. Kapon, Nucleic Acids Res. 2005, 33, 6515.
N. Fardian-Melamed, G. Eidelshtein, D. Rotem, A. Kotlyar, D. Porath, Adv. Mater. 2019, 31, 1902816.
N. Fardian-Melamed, L. Katrivas, G. Eidelshtein, D. Rotem, A. Kotlyar, D. Porath, Nano Lett. 2020, 20, 4505.
G. Eidelshtein, N. Fardian-Melamed, V. Gutkin, D. Basmanov, D. Klinov, D. Rotem, Y. Levi-Kalisman, D. Porath, A. Kotlyar, Adv. Mater. 2016, 28, 4839.
E. Shapir, L. Sagiv, N. Borovok, T. Molotski, A. B. Kotlyar, D. Porath, J. Phys. Chem. B 2008, 112, 9267.
I. Roger-Eitan, K. Liu, G. I. Livshits, N. Borovok, D. Rotem, A. B. Kotlyar, D. Porath, J. Phys. Chem. C 2013, 117, 22462.
W. J. Chung, B. Heddi, E. Schmitt, K. W. Lim, Y. Mechulam, A. T. Phan, Proc. Natl. Acad. Sci. USA 2015, 112, 2729.
N. Fardian-Melamed, G. Eidelshtein, D. Rotem, A. Kotlyar, D. Porath, Small 2019, 16, 1905901.
E. Shapir, H. Cohen, N. Borovok, A. B. Kotlyar, D. Porath, J. Phys. Chem. B 2006, 110, 4430.
E. Shapir, G. Brancolini, T. Molotsky, A. B. Kotlyar, R. Di Felice, D. Porath, Adv. Mater. 2011, 23, 4290.
D. Allison, L. Bottomley, T. Thundat, G. Brown, R. Woychik, J. Schrick, K. B. Jacobson, R. Warmack, Proc. Natl. Acad. Sci. USA 1992, 89, 10129.
L. Bottomley, J. Haseltine, D. Allison, R. Warmack, T. Thundat, R. Sachleben, G. Brown, R. Woychik, K. B. Jacobson, T. Ferrell, J. Vac. Sci. Technol., A 1992, 10, 591.
I. Horcas, R. Fernández, J. Gomez-Rodriguez, J. Colchero, J. Gómez-Herrero, A. Baro, Rev. Sci. Instrum. 2007, 78, 013705.

Auteurs

Liat Katrivas (L)

Department of Biochemistry and Molecular Biology, George S. Wise Faculty of Life Sciences, and, The Center of Nanoscience and Nanotechnology, Tel Aviv University, Ramat Aviv, Tel Aviv, 69978, Israel.

Natalie Fardian-Melamed (N)

Institute of Chemistry and The Center for Nanoscience and Nanotechnology, The Hebrew University of Jerusalem, Jerusalem, 91904, Israel.

Dvir Rotem (D)

Institute of Chemistry and The Center for Nanoscience and Nanotechnology, The Hebrew University of Jerusalem, Jerusalem, 91904, Israel.

Danny Porath (D)

Institute of Chemistry and The Center for Nanoscience and Nanotechnology, The Hebrew University of Jerusalem, Jerusalem, 91904, Israel.

Alexander Kotlyar (A)

Department of Biochemistry and Molecular Biology, George S. Wise Faculty of Life Sciences, and, The Center of Nanoscience and Nanotechnology, Tel Aviv University, Ramat Aviv, Tel Aviv, 69978, Israel.

Articles similaires

DNA Methylation Humans DNA Animals Machine Learning
DNA Glycosylases Nucleosomes Humans 8-Hydroxy-2'-Deoxyguanosine DNA Repair
Alleles Benchmarking Transcription Factors Humans Chromatin Immunoprecipitation Sequencing
Cryoelectron Microscopy Models, Molecular RNA DNA Nucleic Acid Conformation

Classifications MeSH