DFT-Based Stereochemical Rationales for the Bifunctional Brønsted Acid/Base-Catalyzed Diastereodivergent and Enantioselective aza-Henry Reactions of α-Nitro Esters.


Journal

The Journal of organic chemistry
ISSN: 1520-6904
Titre abrégé: J Org Chem
Pays: United States
ID NLM: 2985193R

Informations de publication

Date de publication:
05 11 2021
Historique:
pubmed: 21 10 2021
medline: 27 1 2022
entrez: 20 10 2021
Statut: ppublish

Résumé

A pair of chiral bis(amidine) [BAM] proton complexes provide reagent (catalyst)-controlled, highly diastereo- and enantioselective direct aza-Henry reactions leading to α-alkyl-substituted α,β-diamino esters. A

Identifiants

pubmed: 34669416
doi: 10.1021/acs.joc.1c02112
pmc: PMC8899924
mid: NIHMS1781822
doi:

Substances chimiques

Acids 0
Esters 0
Indicators and Reagents 0

Types de publication

Journal Article Research Support, N.I.H., Extramural Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

15606-15617

Subventions

Organisme : NIGMS NIH HHS
ID : R01 GM084333
Pays : United States

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Auteurs

Thomas J Struble (TJ)

Department of Chemistry and Vanderbilt Institute of Chemical Biology, Vanderbilt University, Nashville, Tennessee 37235, United States.

Ivor Smajlagic (I)

Department of Chemistry, Brock University, 1812 Sir Isaac Brock Way, St. Catharines, Ontario L2S 3A1, Canada.

Hayden Foy (H)

Department of Chemistry, Brock University, 1812 Sir Isaac Brock Way, St. Catharines, Ontario L2S 3A1, Canada.

Travis Dudding (T)

Department of Chemistry, Brock University, 1812 Sir Isaac Brock Way, St. Catharines, Ontario L2S 3A1, Canada.

Jeffrey N Johnston (JN)

Department of Chemistry and Vanderbilt Institute of Chemical Biology, Vanderbilt University, Nashville, Tennessee 37235, United States.

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