Electron Transfer Mechanism at the Interface of Multi-Heme Cytochromes and Metal Oxide.


Journal

Advanced science (Weinheim, Baden-Wurttemberg, Germany)
ISSN: 2198-3844
Titre abrégé: Adv Sci (Weinh)
Pays: Germany
ID NLM: 101664569

Informations de publication

Date de publication:
10 2023
Historique:
received: 26 04 2023
medline: 23 10 2023
pubmed: 17 8 2023
entrez: 17 8 2023
Statut: ppublish

Résumé

Electroactive microbial cells have evolved unique extracellular electron transfer to conduct the reactions via redox outer-membrane (OM) proteins. However, the electron transfer mechanism at the interface of OM proteins and nanomaterial remains unclear. In this study, the mechanism for the electron transfer at biological/inorganic interface is investigated by integrating molecular modeling with electrochemical and spectroscopic measurements. For this purpose, a model system composed of OmcA, a typical OM protein, and the hexagonal tungsten trioxide (h-WO

Identifiants

pubmed: 37587775
doi: 10.1002/advs.202302670
pmc: PMC10582406
doi:

Substances chimiques

Heme 42VZT0U6YR
Bacterial Outer Membrane Proteins 0
Cytochromes 0
Oxides 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2302670

Subventions

Organisme : National Natural Science Foundation of China
ID : 52022093
Organisme : National Natural Science Foundation of China
ID : 51978637
Organisme : National Natural Science Foundation of China
ID : 52192684
Organisme : National Natural Science Foundation of China
ID : 52000166
Organisme : National Natural Science Foundation of China
ID : 51821006
Organisme : Changjiang Scholars Program
Organisme : Innovative Research Team in University of the Ministry of Education of China
Organisme : Youth Innovation Promotion Association
Organisme : USTC Research Funds of the Double First-Class Initiative
ID : YD3530002001
Organisme : Fundamental Research Funds for the Central Universities
ID : WK2400000004

Informations de copyright

© 2023 The Authors. Advanced Science published by Wiley-VCH GmbH.

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Auteurs

Sheng-Song Yu (SS)

Department of Environmental Science and Engineering, University of Science and Technology of China, Hefei, 230026, China.

Xin-Yu Zhang (XY)

Department of Environmental Science and Engineering, University of Science and Technology of China, Hefei, 230026, China.

Shi-Jie Yuan (SJ)

State Key Laboratory of Pollution Control and Resource Reuse, College of Environmental Science and Engineering, Tongji University, Shanghai, 200092, China.

Shen-Long Jiang (SL)

Department of Chemical Physics, University of Science and Technology of China, Hefei, 230026, China.

Qun Zhang (Q)

Department of Chemical Physics, University of Science and Technology of China, Hefei, 230026, China.

Jie-Jie Chen (JJ)

Department of Environmental Science and Engineering, University of Science and Technology of China, Hefei, 230026, China.

Han-Qing Yu (HQ)

Department of Environmental Science and Engineering, University of Science and Technology of China, Hefei, 230026, China.

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Classifications MeSH