Chemical Mimics of Aspartate-Directed Proteases: Predictive and Strictly Specific Hydrolysis of a Globular Protein at Asp-X Sequence Promoted by Polyoxometalate Complexes Rationalized by a Combined Experimental and Theoretical Approach.


Journal

Chemistry (Weinheim an der Bergstrasse, Germany)
ISSN: 1521-3765
Titre abrégé: Chemistry
Pays: Germany
ID NLM: 9513783

Informations de publication

Date de publication:
13 Nov 2019
Historique:
received: 11 06 2019
revised: 13 08 2019
pubmed: 31 8 2019
medline: 21 11 2019
entrez: 31 8 2019
Statut: ppublish

Résumé

Creating efficient and residue-directed artificial proteases is a challenging task due to the extreme inertness of the peptide bond, combined with the difficulty of achieving specific interactions between the catalysts and the protein side chains. Herein we report strictly site-selective hydrolysis of a multi-subunit globular protein, hemoglobin (Hb) from bovine blood, by a range of Zr

Identifiants

pubmed: 31469197
doi: 10.1002/chem.201902675
doi:

Substances chimiques

Coordination Complexes 0
Hemoglobins 0
Tungsten Compounds 0
polyoxometalate I 0
Aspartic Acid 30KYC7MIAI
Zirconium C6V6S92N3C
Peptide Hydrolases EC 3.4.-

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

14370-14381

Subventions

Organisme : KU Leuven
ID : OT/13/060

Informations de copyright

© 2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

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Auteurs

Hong Giang T Ly (HGT)

Laboratory of Bioinorganic Chemistry, Department of Chemistry, KU Leuven, Celestijnenlaan 200F, 3001, Leuven, Belgium.

Tzvetan T Mihaylov (TT)

Laboratory of Computational Coordination Chemistry, Department of Chemistry, KU Leuven, Celestijnenlaan 200F, 3001, Leuven, Belgium.

Paul Proost (P)

Laboratory of Molecular Immunology, Rega Institute, Department of Microbiology, Immunology, and Transplantation, KU Leuven, Herestraat 49, 3000, Leuven, Belgium.

Kristine Pierloot (K)

Laboratory of Computational Coordination Chemistry, Department of Chemistry, KU Leuven, Celestijnenlaan 200F, 3001, Leuven, Belgium.

Jeremy N Harvey (JN)

Laboratory of Computational Coordination Chemistry, Department of Chemistry, KU Leuven, Celestijnenlaan 200F, 3001, Leuven, Belgium.

Tatjana N Parac-Vogt (TN)

Laboratory of Bioinorganic Chemistry, Department of Chemistry, KU Leuven, Celestijnenlaan 200F, 3001, Leuven, Belgium.

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