N-glycome analysis detects dysglycosylation missed by conventional methods in SLC39A8 deficiency.


Journal

Journal of inherited metabolic disease
ISSN: 1573-2665
Titre abrégé: J Inherit Metab Dis
Pays: United States
ID NLM: 7910918

Informations de publication

Date de publication:
11 2020
Historique:
received: 24 06 2020
revised: 07 08 2020
accepted: 26 08 2020
pubmed: 28 8 2020
medline: 8 10 2021
entrez: 28 8 2020
Statut: ppublish

Résumé

Congenital disorders of glycosylation (CDG) are a growing group of inborn metabolic disorders with multiorgan presentation. SLC39A8-CDG is a severe subtype caused by biallelic mutations in the manganese transporter SLC39A8, reducing levels of this essential cofactor for many enzymes including glycosyltransferases. The current diagnostic standard for disorders of N-glycosylation is the analysis of serum transferrin. Exome and Sanger sequencing were performed in two patients with severe neurodevelopmental phenotypes suggestive of CDG. Transferrin glycosylation was analyzed by high-performance liquid chromatography (HPLC) and isoelectric focusing in addition to comprehensive N-glycome analysis using matrix-assisted laser desorption ionization time of flight (MALDI-TOF) mass spectrometry (MS). Atomic absorption spectroscopy was used to quantify whole blood manganese levels. Both patients presented with a severe, multisystem disorder, and a complex neurological phenotype. Magnetic resonance imaging (MRI) revealed a Leigh-like syndrome with bilateral T2 hyperintensities of the basal ganglia. In patient 1, exome sequencing identified the previously undescribed homozygous variant c.608T>C [p.F203S] in SLC39A8. Patient 2 was found to be homozygous for c.112G>C [p.G38R]. Both individuals showed a reduction of whole blood manganese, though transferrin glycosylation was normal. N-glycome using MALDI-TOF MS identified an increase of the asialo-agalactosylated precursor N-glycan A2G1S1 and a decrease in bisected structures. In addition, analysis of heterozygous CDG-allele carriers identified similar but less severe glycosylation changes. Despite its reliance as a clinical gold standard, analysis of transferrin glycosylation cannot be categorically used to rule out SLC39A8-CDG. These results emphasize that SLC39A8-CDG presents as a spectrum of dysregulated glycosylation, and MS is an important tool for identifying deficiencies not detected by conventional methods.

Identifiants

pubmed: 32852845
doi: 10.1002/jimd.12306
pmc: PMC8086894
mid: NIHMS1692330
doi:

Substances chimiques

Cation Transport Proteins 0
SLC39A8 protein, human 0
Transferrin 0
Manganese 42Z2K6ZL8P

Types de publication

Journal Article Multicenter Study Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

1370-1381

Subventions

Organisme : NIMH NIH HHS
ID : T32 MH112485
Pays : United States

Informations de copyright

© 2020 The Authors. Journal of Inherited Metabolic Disease published by John Wiley & Sons Ltd on behalf of SSIEM.

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Auteurs

Julien H Park (JH)

Department of Clinical Sciences, Neurosciences, Umeå University, Umeå, Sweden.
Department of General Pediatrics, University of Münster, Münster, Germany.

Robert G Mealer (RG)

Psychiatric and Neurodevelopmental Genetics Unit, Massachusetts General Hospital, Harvard Medical School, Boston, Massachusetts, USA.
The Stanley Center for Psychiatric Research at Broad Institute of Harvard/MIT, Cambridge, Massachusetts, USA.
National Center for Functional Glycomics, Department of Surgery, Beth Israel Deaconess Medical Center, Harvard Medical School, Boston, Massachusetts, USA.

Abdallah F Elias (AF)

Department of Medical Genetics, Shodair Children's Hospital, Helena, Montana, USA.
Division of Medical Genetics, Department of Pediatrics, University of Utah, Salt Lake City, Utah, USA.

Susanne Hoffmann (S)

Zentrum für Sozial- und Neuropädiatrie, Vivantes Klinikum Neukölln, Berlin, Germany.

Marianne Grüneberg (M)

Department of General Pediatrics, University of Münster, Münster, Germany.

Saskia Biskup (S)

CeGAT GmbH and Praxis für Humangenetik Tübingen, Tübingen, Germany.

Manfred Fobker (M)

Center for Laboratory Medicine, University Hospital Münster, Münster, Germany.

Jaclyn Haven (J)

Department of Medical Genetics, Shodair Children's Hospital, Helena, Montana, USA.

Ute Mangels (U)

Department of General Pediatrics, University of Münster, Münster, Germany.

Janine Reunert (J)

Department of General Pediatrics, University of Münster, Münster, Germany.

Stephan Rust (S)

Department of General Pediatrics, University of Münster, Münster, Germany.

Jonathan Schoof (J)

Department of Medical Genetics, Shodair Children's Hospital, Helena, Montana, USA.

Corbin Schwanke (C)

Department of Medical Genetics, Shodair Children's Hospital, Helena, Montana, USA.

Jordan W Smoller (JW)

Psychiatric and Neurodevelopmental Genetics Unit, Massachusetts General Hospital, Harvard Medical School, Boston, Massachusetts, USA.
The Stanley Center for Psychiatric Research at Broad Institute of Harvard/MIT, Cambridge, Massachusetts, USA.

Richard D Cummings (RD)

National Center for Functional Glycomics, Department of Surgery, Beth Israel Deaconess Medical Center, Harvard Medical School, Boston, Massachusetts, USA.

Thorsten Marquardt (T)

Department of General Pediatrics, University of Münster, Münster, Germany.

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Classifications MeSH