High-throughput and reliable assessments of the ionization constant of monoprotic organic acids through an arginine based mixed mode HPLC.


Journal

Journal of pharmaceutical and biomedical analysis
ISSN: 1873-264X
Titre abrégé: J Pharm Biomed Anal
Pays: England
ID NLM: 8309336

Informations de publication

Date de publication:
25 Oct 2023
Historique:
received: 08 06 2023
revised: 19 07 2023
accepted: 24 07 2023
medline: 11 9 2023
pubmed: 3 8 2023
entrez: 2 8 2023
Statut: ppublish

Résumé

The charge state of a molecule is the single most prominent attribute ruling out its interactions with the surrounding environment. In a previous study, the retention of acids on the new Celeris™ Arginine (ARG) column was found to be predominantly driven by electrostatics and, specifically, their charge state. Therefore, we analysed 41 compounds in liquid chromatography with ultraviolet detection to study possible relationships between the analytical retention on this phase and the pK

Identifiants

pubmed: 37531733
pii: S0731-7085(23)00373-4
doi: 10.1016/j.jpba.2023.115604
pii:
doi:

Substances chimiques

Arginine 94ZLA3W45F
Organic Chemicals 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

115604

Informations de copyright

Copyright © 2023 The Authors. Published by Elsevier B.V. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of Competing Interest The authors declare the following financial interests/personal relationships which may be considered as potential competing interests: Scott Anderson was the Scientific Director of Regis Technologies Inc., that developed and manufactured the Celeris™ Arginine column, whose application is described in the present study.

Auteurs

Giacomo Russo (G)

School of Applied Sciences, Sighthill Campus, Edinburgh Napier University, 9 Sighthill Ct, EH11 4BN Edinburgh, United Kingdom. Electronic address: g.russo@napier.ac.uk.

Ardiana Kajtazi (A)

Separation Science Group, Department of Organic and Macromolecular Chemistry, Ghent University, Krijgslaan 281 S4bis, B-9000 Ghent, Belgium.

Maura Vallaro (M)

CASSMedChem Research Group, Molecular Biotechnology and Health Sciences Department, University of Turin, piazza Nizza 44 bis 10126 Turin, Italy.

Pieter Surmont (P)

Separation Science Group, Department of Organic and Macromolecular Chemistry, Ghent University, Krijgslaan 281 S4bis, B-9000 Ghent, Belgium.

Giuseppe Ermondi (G)

CASSMedChem Research Group, Molecular Biotechnology and Health Sciences Department, University of Turin, piazza Nizza 44 bis 10126 Turin, Italy.

Scott Anderson (S)

Regis Technologies Inc., 8210 Austin Ave, Morton Grove, IL 60053, USA.

Lucia Grumetto (L)

Department of Pharmacy, School of Medicine and Surgery, University of Naples Federico II, Via D. Montesano, 49, I-80131 Naples, Italy.

Giulia Caron (G)

CASSMedChem Research Group, Molecular Biotechnology and Health Sciences Department, University of Turin, piazza Nizza 44 bis 10126 Turin, Italy.

Frédéric Lynen (F)

Separation Science Group, Department of Organic and Macromolecular Chemistry, Ghent University, Krijgslaan 281 S4bis, B-9000 Ghent, Belgium.

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Classifications MeSH